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Integer-order calculus fails to capture the long-range dependence (LRD) and memory effects found in many complex systems. Fractional calculus addresses these gaps through fractional-order integrals and derivatives, but fractional-order dynamical systems pose substantial challenges in system identification and optimal control tasks. In this paper, we theoretically derive the optimal control via linear quadratic regulator (LQR) for fractional-order linear time-invariant (FOLTI) systems and develop an end-to-end deep learning framework based on this theoretical foundation. Our approach establishes a rigorous mathematical model, derives analytical solutions, and incorporates deep learning to achieve data-driven optimal control of FOLTI systems. Our key contributions include: (i) proposing a novel method for system identification and optimal control strategy in FOLTI systems, (ii) developing the first end-to-end data-driven learning framework, Fractional-Order Learning for Optimal Control (FOLOC), that learns control policies from observed trajectories, and (iii) deriving theoretical bounds on the sample complexity for learning accurate control policies under fractional-order dynamics. Experimental results indicate that our method accurately approximates fractional-order system behaviors without relying on Gaussian noise assumptions, pointing to promising avenues for advanced optimal control.